<< 5. Neutral Detergent Fiber - Amylase Procedure

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5.1 Determination of Amylase Neutral Detergent Fiber by Refluxing

Reference:
Goering, H.K. and P.J. Van Soest. 1970. Forage fiber analysis (apparatus, reagents, procedures, and some applications). USDA Agricultural Research Service. Handbook number 379 as modified by D.R. Mertens (1992, Personal Communication).

Van Soest, P.J, J.B. Robertson, and B.A. Lewis. 1991. Methods for dietary fiber, neutral detergent fiber and non-starch polysaccharides in relation to animal nutrition. J. Dairy Science 74:3583-3597.

Mertens, D.R. 1992. Critical conditions in determining detergent fiber. Proceedings of NFTA Forage Analysis Workshop. Denver, CO. p C1-C8.

Scope:
This method is applicable for the determination of neutral detergent fiber in all types of forages and feeds.

Basic Principle:
A neutral detergent solution is used to dissolve the easily digested pectins and plant cell contents (proteins, sugars and lipids), leaving a fibrous residue (aNDF) that is primarily cell wall components of plants (cellulose, hemicellulose and lignin). Detergent is used to solubilize the proteins and sodium sulfite also helps remove some nitrogenous matter; EDTA is used to chelate calcium and remove pectins at boiling temperatures; triethylene glycol helps to remove some nonfibrous matter from concentrate feeds; and heat-stable amylase is used to remove starch. Two additions of amylase (one during refluxing and one during filtration) have been observed to aid aNDF analyses and minimize filtering difficulties. Heat-stable amylases are used in hot solutions to inactivate potential contaminating enzymes that might degrade fibrous constituents.

Equipment: Refluxing apparatus
Berzelius beakers (600 mL)
Fritted glass (Gooch) crucibles (coarse porosity, 50 mL)
Analytical electronic balance, accurate to 0.1 mg
Suction filtering device with trap in line and
valve to break vacuum Forced-air drying oven set at 100oC

Reagents:
Neutral detergent solution - To make approximately 18 liters mix:
17.82 L Distilled water 540 g Sodium lauryl sulfate, USP 335 g Ethylenediami netetraacetic acid (EDTA), disodium salt (may substitute 72 g sodium hydroxide (NaOH) and 263 g free acid EDTA as a less expensive alternative.)

122.6 g Sodium borate, decahydrate (Na2B4O7.10H2O), reagent grade 82.1 g Sodium phosphate, dibasic (Na2HPO4), anhydrous, reagent grade 180 mL Triethylene glycol, reagent grade

Preparing a NDF Solution
Pour one-half of distilled water into mixing container. Place on stir plate in hood and begin stirring. Add remaining reagents except for triethylene glycol. (Caution: wear dust mask when weighing and transferring the sodium lauryl sulfate.) Slowly add remaining distilled water to container to limit foaming of the detergent. When approximately three-fourths of the distilled water has been added to the container, add the triethylene glycol. The triethylene glycol will reduce foaming of the detergent solution. Allow to stir overnight. Use heated stirrer if material fails to dissolve. Keep container at 20oC or higher to avoid precipitation of the solution. Verify pH of solution to be between 6.95 and 7.05. Adjust with HCl or NaOH as required if not within range. Reagents, Sodium sulfite, anhydrous (Na2SO3), reagent grade Acetone, reagent grade Heat-stable alpha-amylase solution (standardized by method 5.1.1)

Safety Precautions:

  • Acetone is highly flammable. Do not let vapors accumulate in work area. Use effective fume removal device. Also avoid inhaling or contact with skin. Make sure all traces of acetone have evaporated from crucibles containing the fiber residue before placing them into the oven.
  • Sodium lauryl sulfate is irritating to mucous membranes. Wear dust mask and gloves while handling.

Procedure:

  1. Samples should be microwave or oven dried at 55oC to greater than 85% dry matter, then ground to pass a 1 mm screen.
  2. Dry 50 mL fritted glass crucibles overnight at 100oC and hot weigh (W1), recording weight to nearest 0.1 mg. (Refer to method 2.2.2.2 for description of hot weighing techniques.)
  3. Thoroughly mix sample, then weigh 0.45 to 0.55 g, recording to nearest 0.1 mg, (W2) into 600 mL Berzelius beaker. Weigh a second subsample for laboratory dry matter determination.
  4. Preheat extraction heating (reflux) unit to a temperature that permits boiling of neutral detergent solution within 5 min.
  5. Add 0.5 g of sodium sulfite using previously calibrated scoop.
  6. Add 50 mL of neutral detergent solution and swirl beaker until the sample and sodium sulfite are completely suspended.
  7. Place beaker on the heating unit under a cool water condenser. Samples should come to a boil in 4 to 5 min. Samples normally foam vigorously for 1 to 2 min. Do not reduce temperature of heating unit during this time.
  8. After 5 min, remove beaker from the reflux unit and add 2 mL of the standardized amylase solution.
  9. Swirl beaker to thoroughly mix the amylase in the neutral detergent solution and resuspend any particles that have crept up the sides of the beaker. Detach any sample attached to the sides or bottom of the beaker using a rubber policeman. Rinse off policeman with aNDF solution.
  10. Return beaker to the reflux unit and allow to come to a boil. Reflux for 60 min. Five to 10 min after adding amylase, rinse down the sides of the beaker with neutral detergent solution.
  11. Remove sample from heating unit and allow to settle for 30-60 sec before filtering.
  12. Preheat the fritted glass crucible for filtering by adding 40 mL of boiling water. Remove water with vacuum.
  13. Carefully decant the first 30-40 mL of solution from the Berzelius beaker into the crucible. Rinse lip of beaker to prevent solution with particles from running down outside of beaker. Keep beaker in "decant" position while emptying. Remove the solution with a minimum amount of vacuum.
  14. Close vacuum and rinse the remaining residue from the beaker into the crucible using a fine stream of boiling water. Be certain that no particles remain in the beaker or on the lip to run down the outside as the beaker is turned upright. Apply minimum vacuum to filter.
  15. Immediately fill crucible half full of hot water and add 2 mL of standardized amylase solution. Allow to react for approximately 45 to 60 sec, while policing particles from sides of Berzelius beaker.
  16. Rinse Berzelius beaker with boiling water while inverted over the crucible until all residue is transferred.
  17. Filter and wash twice by adding 30 to 40 mL boiling water to residue in fritted glass crucible and allowing to soak for 2 min each time.
  18. Rinse sample twice with 30 mL of acetone, allowing at least 2 min soaking time between rinses.
  19. Rinse policeman, vacuum sample dry, and remove sample from manifold.
  20. Dry crucibles at 100oC for 8 hr or overnight and hot weigh recording weight (W3) to nearest 0.1 mg.

Comments:

  • Difficult filtration may result from plugging of the fritted glass crucibles. Crucibles should be cleaned regularly with acid or alkaline cleaning solution. The filtration rate of crucibles should be as uniform as possible for a given set of samples. To check the filtration rate of crucibles, fill them with 50 mL of distilled water and record the time required to drain completely without vacuum. This should be about 180 sec. If filtration takes more than 240 sec, crucibles need cleaning. If cleaning does not improve the filtration rate, the crucible should be discarded. If filtering takes less than 120 sec, check crucible for cracks or holes in the fritted disk. If filtering takes less than 100 sec, the crucible should be discarded.
  • The proper vacuum is critical to good filtering. It should be sufficient to remove the solutions rapidly but not so great that fiber particles plug the fritted glass disc.
  • Rinse water must be in excess of 95oC. This is particularly true for samples containing pectic substances, mucilages or glycoproteins.
  • Some sample types are consistently difficult to filter (corn silage, citrus pulp, sunflower meal, meat by-products and feces). Experience has shown that any sample that takes longer than 10 min to filter will provide erroneous results and must be repeated using modifications described by Mertens or Van Soest.
  • Many amylase extracts are crude mixtures that may contain fiber degrading enzymes. Because heat will inactivate these contaminating enzymes, it is recommended that a heat-stable amylase be used in hot solution to minimize fiber loss.

Calculation: Percent Amylase Neutral Detergent Fiber (aNDF)

aNDF (DM basis) = W3 - W1 / W2 X Lab DM / 100 X 100

  • W1 = tare weight of crucible in grams
  • W2 = initial sample weight in grams
  • W3 = dry weight of crucible and dry fiber in grams

Quality Control:
Include one or more quality control (QC) samples in each run, choosing QC samples by matching analyte levels and matrices of QC samples to the samples in the run. Include at least one set of duplicates in each run if single determinations are being made.

An acceptable average standard deviation among replicated analyses for neutral detergent fiber ranges from about ±0.35 for samples with 40% NDF to ±0.60 for samples with 70% NDF, which results in warning limits (2s) ranging from ±0.70 to 1.20 and control limits (3s) ranging from ±1.05 to 1.80. Plot the results of the control sample(s) on an X-control chart and examine the chart for trends. Results outside of upper or lower warning limits, ±2s (95 percent confidence limits), are evidence of possible problems with the analytical system. Results outside of upper or lower control limits, ±3s (99 percent confidence limits), indicate loss of control and results of the run should be discarded. Two consecutive analyses falling on one side of the mean between the warning limits and the control limits also indicate loss of control.

 

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